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化学反应与工程研究组
催化反应与过程强化组
低碳清洁能源研究组
环境与能源功能材料组
矿物绿色加工研究组
能源化工与碳减排研究组
先进材料工程化研究组
材料表界面与传质强化组
资源与环境微生物实验室

环境与能源先进功能材料研究组

 

 


小组简介：

欢迎来到环境与能源先进材料研究组！

本研究组共有教授1名、副教授1名、博士后1名、博士研究生8名和硕士研究生19名。研究组主要围绕环境与能源先进材料开展研究，耦合新工艺开发及反应、分离过程强化开展成果转化，具体领域包括：超浸润材料及油水分离、防腐新技术、气体净化（NH3、H2S、SO2、CO、挥发性有机物等）、CO2捕集及催化转化、电化学储能、固废循环资源化等。研究组致力于通过先进功能材料的理性设计、可控制备、结构性质及反应机理研究，解决环境污染及能源匮乏的问题。课题组拥有齐全的实验仪器，包括气相色谱、质谱仪、电化学工作站、CO2静态/动态吸附仪、热/光/电催化反应器（间歇及半连续反应器、微型固定床反应器）、紫外可见分光光度仪、接触角测量仪、四探针测量仪、冷冻干燥机等，为研究开展提供了强有力的支撑。

研究团队：

袁绍军

邮箱：

ysj@scu.edu.cn                  

职位：

教授

联系电话：

028-85405201

 

欧阳李科

邮箱：

Like.ouyang@scu.edu.cn

职位：

副教授

联系电话：

 

王缘

邮箱：

wangyuan2022@scu.edu.cn

职位：

副研究员

联系电话：

 

贺革

邮箱：

hege@scu.edu.cn

职位：

助理研究员

联系电话：

 

 

研究方向：

1、多孔碳用于CO2捕集和电化学储能

针对温室效应和能源危机，开展了新型绿色碳基纳米多孔材料的设计和制备以缓解CO2捕集和电化学储能问题。包括：1、杂原子（N、P、S）掺杂多孔碳的设计和可控制备；2、杂原子掺杂多孔碳基柔性电极的制备及其在电化学储能中的应用；3、MOFs复合杂原子掺杂生物质碳基吸附剂的制备及其在CO2和NH3吸附中的应用。

2、光/电催化剂设计及污染物去除

采用光/电催化技术对地下水中砷、铬等重金属离子和有机污染物实现有效去除，通过设计TiO2等半导体光催化剂，以及IrO2、RuO2等Ti基复合金属氧化物电极在光照或外加电场的作用下实现有机污染物和重金属离子降解和氧化，为地下水资源的保护和净化提供了一种可行的解决方案，并进一步优化催化剂的性能和反应条件，提高光/电催化技术在地下水污染处理中的应用效果，促进环境保护和可持续发展。

3、超浸润材料与油水分离和防腐应用

含油废水是水污染的主要来源之一。受仿生学启发，具有特殊浸润性的膜材料（超疏水/超亲油性或超亲水/水下超疏油性等）是具有良好发展前景的绿色高效分离技术。本课题组通过简便易放大的制备技术（如化学刻蚀、溶剂热、层层自组装、和静电纺丝等）为基础，以膜表面污染防治、乳液分离过程强化、按需乳液分离切换等科学问题为导向，精确设计了多种特殊浸润性网膜，并在油水乳液分离领域取得了一定的研究进展。

4、吸附催化新材料及气体净化

VOCs和恶臭气体排放日益增多，对自然环境和人类生存带来了巨大的威胁。团队利用吸附-催化耦合法和光催化法在消减气相典型污染物研究领域中取得了重要进展。开发了一系列以废弃生物质为原料负载金属氧化物的高选择性脱硫脱氨剂，以及以TiO2纳米颗粒为基底构建Z型异质结的高效光催化剂，具有广泛的应用价值。

5、催化剂设计及合成氨应用

氨是现代工业及农业化肥的重要原料，也是氢能的主要载体。在常温常压下将硝酸盐废水电催化还原为氨（NO3RR），对于解决环境问题且兼顾经济效益具有重要意义。团队主要针对过渡金属及其合金、氧化物、磷化物等材料进行设计，提高反应活性和选择性。

代表性项目：

1、国家重点研发计划“固废资源化”课题，2019YFC1900604，城乡混合有机垃圾好氧发酵副产物风险控制及可持续利用技术与装备，2020.12-2023.12，负责人

2、国家自然科学基金面上项目，21978182，填充式钛基纳米复合涂层电极的可控制备与电催化氧化-吸附耦合除砷机理， 2020.01-2023.12，负责人

3、国家自然科学基金面上项目，21676169，磁载导电聚合物/TiO2纳米复合材料可控制备与光催化氧化-吸附协同除砷机理，2017.01-2020.12，负责人

4、国家重点研发计划子课题，2016YFB0301701，多相氧化组合反应器数值放大与耦合强化，2016.07-2021.06，负责人

5、微纳米含氮导电聚合物吸附脱碳技术研究，2016.01-2018.12，中国石油化工股份有限公司，负责人

近三年发表文章：

  1. Xinyu Miao, Jiao Shen, Wenlan Ji, Tian C Zhang, Ying Liang, Shaojun Yuan*, Boosting electrochemical oxidation of As(III) on Fe-doped RuO2/PEDOT/SnO2 nanocomposite anode: Fabrication, performance and mechanism, Journal of Materials Science & Technology 180 (2024), 243-258.

  2. Wenlan Ji, Weiwei Li, Yuan Wang, Tian C Zhang, Shaojun Yuan*, Fe-MOFs/graphene oxide-derived magnetic nanocomposite for enhanced adsorption of As(V) in aqueous solution, Separation and Purification Technology 334 (2024) 126003.

  3. Yi Yuan, Genghua Wu, Weikeduo Li, Yuan Wang, Tian C Zhang, Ge He, Shaojun Yuan*, In situ growth of MIL-100 (Fe) onto the rice straw-derived biochar for efficient adsorption of gaseous ammonia, Separation and Purification Technology, 242 (2024) 127034.

  4. Quyun Chen, Yuan Wang, Ge He, Murat Yilmaz, Shaojun Yuan*, KMnO4-activated spinach waste biochar: An efficient adsorbent for adsorption of heavy metal ions in aqueous solution, Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2024, 684, 133174.

  5. Yajie Liu, Yuan Wang, Tian C Zhang, Like Ouyang, Shaojun Yuan*, Switchable superlyophobic PAN@ Co-MOF membrane for on-demand emulsion separation and efficient soluble dye degradation, Separation and Purification Technology, 2024, 331, 125730.

  6. Yanxu Wang, Lijia Huang, Tian C Zhang, Yan Wang, Shaojun Yuan*, Visible-Light-Induced photocatalytic oxidation of gaseous ammonia on Mo, c-codoped TiO2: Synthesis, performance and mechanism, Chemical Engineering Journal, 2024, 482, 148811.

  7. Wenlan Ji, Weiwei Li, Yuan Wang, Tian C Zhang, Yibin Wei, Shaojun Yuan*, Zr-doped MIL-101 (Fe)/graphene oxide nanocomposites: An efficient and water-stable MOF-based adsorbent for As(V) adsorption in aqueous solution, Separation and Purification Technology, 2023, 339, 126681.

  8. Yuan Wang, Tao Zhang, Xuelian Zheng, Xiaobao Tian, Shaojun Yuan*, Enhancing energy storage via confining sulfite anions onto iron oxide/poly (3, 4-ethylenedioxythiophene) heterointerface, ACS Applied Materials & Interfaces, 2023, 15 (51), 59413-59421.

  9. Huaqiang He, Haoran Ma, Yajie Liu, Tian C Zhang, Shaojun Yuan*, A biomimetic superwetting Bi2MoO6-dotted PAA/CS@ CuC2O4 membrane with self-cleaning and self-healing ability to aggregate oil droplets for enhanced demulsification of O/W emulsion, Materials Today Nano, 2023, 24, 100426.

  10. Jianfei Xiao, Yufang Zhang, Tian C Zhang, Yuan Wang, Shaojun Yuan*, Cu3BTC2 MOF-impregnated boron-doped biochar derived from orange peels for enhanced NH3 capture, Applied Surface Science, 2023, 635, 157735.

  11. Yi Yuan, Lijia Huang, Tian C Zhang, Yuan Wang, Shaojun Yuan*, CaCO3-ZnO loaded scrap rice-derived biochar for H2S removal at room-temperature: Characterization, performance and mechanism, Fuel Processing Technology, 2023, 249, 107846.

  12. Yue Wu, Guangyuan Lu, Ping Xu, Tian C Zhang, Huaqiang He, Shaojun Yuan*, Hierarchical Ni-Mn LDHs@ CuC2O4 nanosheet arrays-modified copper mesh: A dual-functional material for enhancing oil/water separation and supercapacitors, International Journal of Molecular Sciences, 2023, 24 (18), 14085.

  13. Yuyi Liao, Zhongtao Shang, Guangrui Ju, Dingke Wang, Qiao Yang, Yuan Wang, Shaojun Yuan*, Biomass derived N-doped porous carbon made from reed straw for an enhanced supercapacitor, Molecules, 2023, 28 (12), 4633.

  14. Yajie Liu, Huaqiang He, Tie-Jun Zhang, Tian C Zhang, Yuan Wang, Shaojun Yuan*, A biomimetic beetle-like membrane with superoleophilic SiO2-induced oil coalescence on superhydrophilic CuC2O4 nanosheet arrays for effective O/W emulsion separation, Journal of Hazardous Materials, 2023, 451, 131142.

  15. Wenlan Ji, Weiwei Li, Tian C Zhang, Yuan Wang, Shaojun Yuan*, Constructing dimensionally stable TiO2 nanotube arrays/SnO2/RuO2 anode via successive electrodeposition for efficient electrocatalytic oxidation of As(III), Separation and Purification Technology, 2023, 312, 123370.

  16. Wenlan Ji, Yijiang He, Tian C Zhang, Yuan Wang, Shaojun Yuan*, Nickel-based non-noble metal layered double hydroxide grown on carbon cloth for boosting electrocatalytic oxidation of As (III), Applied Surface Science, 2023, 618, 156631.

  17. Yi Yuan, Lijia Huang, Murat Yılmaz, Tian C Zhang, Yuan Wang, Shaojun Yuan*, MgFe2O4-loaded N-doped biochar derived from waste cooked rice for efficient low-temperature desulfurization of H2S, Fuel, 2023, 339, 127385.

  18. Yanbo Deng, Lian Fu, Wenjia Song, Like Ouyang, Shaojun Yuan, Transition metal and Pr co-doping induced oxygen vacancy in Pd/CeO2 catalyst boosts low-temperature CO oxidation, Separation and Purification Technology, 2023, 311, 123247.

  19. Lijia Huang, Hui Liu, Yuan Wang, Tian C Zhang, Shaojun Yuan*, Construction of ternary Bi2O3/biochar/g-C3N4 heterojunction to accelerate photoinduced carrier separation for enhanced tetracycline photodegradation, Applied Surface Science, 2023, 616, 156509.

  20. Genghua Wu, Jianfei Xiao, Murat Yılmaz, Tian C Zhang, Shaojun Yuan*, Fusiform CuC2O4 loaded porous biochar derived from phosphoric acid-activated bagasse for gaseous ammonia capture, Journal of Environmental Chemical Engineering, 2023, 11 (2), 109466.

  21. Ying Liu, Baogang Sun, Wenting Jia, Yuan Wang, Lijia Huang, Pengge Ning, Shaojun Yuan, Study on removal mechanism for copper cyanide complex ions in water: Ion species differences and evolution process, International Journal of Molecular Sciences 2023, 24 (6), 5066.

  22. Ji Li, Junfeng Lu, Tian C Zhang, Shaojun Yuan*, Superhydrophobic DTMS/rGO-nanocomposites modified polyurethane sponge for efficient oil-water separation, Surface Engineering, 2023, 39 (3), 349-360.

  23. Weiwei Li, Wenlan Ji, Murat Yılmaz, Tian C Zhang, Shaojun Yuan*, One-Pot synthesis of MWCNTs/Fe-MOFs nanocomposites for enhanced adsorption of As (V) in aqueous solution, Applied Surface Science, 2023, 609, 155304.

  24. Yuan Wang, Tao Zhang, Jianfei Xiao, Xiaobao Tian, Shaojun Yuan*, Enhancing electrochemical performance of ultrasmall Fe2O3-embedded carbon nanotubes via combusting-induced high-valence dopants, Journal of Materials Science & Technology, 2023, 134, 142-150.

  25. Chunhui Wu, Zifan Pei, Menglin Lv, Duchen Huang, Yuan Wang, Shaojun Yuan*, Polypyrrole-coated low-crystallinity iron oxide grown on carbon cloth enabling enhanced electrochemical supercapacitor performance, Molecules, 2023, 28 (1), 434.

  26. Senhao Wang, Yuan Wang, Tian C Zhang, Xu Ji, Shaojun Yuan*, Ti-doped iron phosphide nanoarrays grown on carbon cloth as a self-supported electrode for enhanced electrocatalytic nitrogen reduction, Nanoscale, 2023, 15(39), 16219-16226.

  27. Jianfei Xiao, Yufang Zhang, Tian C Zhang, Shaojun Yuan*, Prussian blue-impregnated waste pomelo peels-derived biochar for enhanced adsorption of NH3, Journal of Cleaner Production, 2023, 382, 135393.

  28. Qi Guo, Tengle Wang, Tian C Zhang, Like Ouyang, Shaojun Yuan*, Superhydrophobic double layered MgAl-LDH/epoxy composite coatings for enhanced anticorrosion performance of magnesium alloys, Progress in Organic Coatings, 2023, 174, 107300.

  29. Yanbo Deng, Shijie Liu, Lian Fu, Yi Yuan, Anmin Zhao, Dajun Wang, Heng Zheng, Like Ouyang, Shaojun Yuan, Crystal plane induced metal-support interaction in Pd/Pr-CeO2 catalyst boosts H2O-assisted CO oxidation, Journal of Catalysis, 2023, 417, 60-73.

  30. Wenlan Ji, Xinyu Miao, Tian C Zhang, Yuan Wang, Shaojun Yuan*, Fe-metal-organic-framework/MnO2 nanowire/granular activated carbon nanostructured composites for enhanced As (III) removal from aqueous solutions, Applied Surface Science, 2022, 606, 155011.

  31. Huaqiang He, Yue Wu, Yuan Wang, Tie-Jun Zhang, Tian C Zhang, Shaojun Yuan*, Constructing A Janus membrane with extremely asymmetric wettability for water unidirectional permeation and switchable emulsion separation, Separation and Purification Technology, 2022, 303, 122254.

  32. Jialing Tang, Hao Yuan, Qiong Duan, Yinan Liu, Yuan Wang, Shaojun Yuan*, Phosphorus-functionalized low-crystallinity transition-metal oxide nanorod arrays grown on carbon cloth for high-performance asymmetric supercapacitors, Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2022, 654, 130189.

  33. Lijia Huang, Yi Yuan, Yuan Wang, Murat Yılmaz, Tian C Zhang, Shaojun Yuan*, Visible-light-driven photocatalytic oxidation of H2S by boron-doped TiO2/LDH heterojunction: synthesis, performance, and reaction mechanism, Chemical Engineering Journal, 2022, 448, 137607.

  34. Xiang Liu, Tian C Zhang, Yuxin Zhang, Jinsong Rao, Shaojun Yuan*, A route for large-scale preparation of multifunctional superhydrophobic coating with electrochemically-modified kaolin for efficient corrosion protection of magnesium alloys, Journal of Magnesium and Alloys, 2022, 10(11), 3082-3099.

  35. Lijia Huang, Hui Liu, Tian Cheng Zhang, Yuan Wang, Shaojun Yuan*, Peroxymonosulfate-assisted BiVO4/exfoliated g-C3N4 heterojunction for high-performance photodegradation of tetracycline induced by visible light. Industrial & Engineering Chemistry Research, 2022, 61(44), 16418-16430.

  36. Xiaofang Yuan, Jianfei Xiao, Murat Yılmaz, Tian C Zhang, Shaojun Yuan*, N, P Co-doped porous biochar derived from cornstalk for high performance CO2 adsorption and electrochemical energy storage, Separation and Purification Technology, 2022, 299, 121719.

  37. Jianfei Xiao, Xiaofang Yuan, Tian C Zhang, Like Ouyang, Shaojun Yuan*, Nitrogen-doped porous carbon for excellent CO2 capture: A novel method for preparation and performance evaluation, Separation and Purification Technology, 2022, 298, 121602.

  38. Thabang Mokoba, Yajie Liu, Yue Wu, Tian Cheng Zhang, Shaojun Yuan*, Agave-angustifolia-like Cu3Mo2O9 nanoplate-coated copper mesh for effective emulsion separation and photocatalytic degradation of soluble dyes, Industrial & Engineering Chemistry Research, 2022, 61(36), 13635-13649.

  39. Tengle Wang, Qi Guo, Tian C Zhang, Yu-Xin Zhang, Shaojun Yuan*, Large-scale prepared superhydrophobic HDTMS-modified diatomite/epoxy resin composite coatings for high-performance corrosion protection of magnesium alloys, Progress in Organic Coatings, 2022, 170, 106999.

  40. Thabang Mokoba, Zhikai Li, Tian C Zhang, Shaojun Yuan*, Superwetting sea urchin-like BiOBr@Co3O4 nanowire clusters-coated copper mesh with efficient emulsion separation and photo-Fenton-like degradation of soluble dye, Applied Surface Science 2022, 594, 153497.

  41. Lian Fu, Shijie Liu, Yanbo Deng, Huaqiang He, Shaojun Yuan, Like Ouyang, Fabrication of the PdAu surface alloy on an ordered intermetallic Au3Cu core for direct H2O2 synthesis at ambient pressure, Industrial & Engineering Chemistry Research, 2022, 61 (32), 11655-11665.

  42. Wenlan Ji, Yuan Wang, Yuanjie Xiong, Tian C Zhang, Shaojun Yuan*, Hydrophobic Ce-doped β-PbO2-SDS anode achieving synergistic effects for enhanced electrocatalytic oxidation of As(III), Separation and Purification Technology, 2022, 294, 121214.

  43. Huaqiang He, Yajie Liu, Yingming Zhu, Tian C Zhang, Shaojun Yuan*, Underoil superhydrophilic CuC2O4@ Cu-MOFs core-shell nanosheets-coated copper mesh membrane for on-demand emulsion separation and simultaneous removal of soluble dye, Separation and Purification Technology, 2022, 293, 121089.

  44. Ji Li, Yuan Wang, Ruixi Gao, Tian C Zhang, Shaojun Yuan*, Superhydrophobic copper foam modified with hierarchical stearic acid/CuSiO3/Cu(OH)2 nanocomposites for efficient water/oil separation, Journal of Environmental Chemical Engineering, 2022, 10 (3), 107618.

  45. Yuan Wang, Xuemei Liu, Quyun Chen, Tian C Zhang, Like Ouyang, Shaojun Yuan*, Simultaneous photocatalytic oxidation and adsorption for efficient As (III) removal by magnetic BiOI/γ-Fe2O3 core–shell nanoparticles, Materials Today Chemistry, 2022, 24, 100823.

  46. Baibing Wei, Kai Wang, Jiarong Wang, Tian C Zhang, Xiaobao Tian, Shaojun Yuan, Yingqi Li, Haiqing Chang, Ying Liang, Zhihong Zhou, Thermo-modulated nanofibrous skin covered Janus membranes for efficient oil/water separation, Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2022, 641, 127935.

  47. Hongxia Li, Aikifa Raza, Shaojun Yuan, Faisal AlMarzooqi, Nicholas X Fang, TieJun Zhang, Biomimetic on-chip filtration enabled by direct micro-3D printing on membrane, Scientific Reports, 2022, 12 (1), 8178.

  48. Wenlan Ji, Yuanjie Xiong, Yuan Wang, Tian C Zhang, Shaojun Yuan*, Multilayered TNAs/SnO2/PPy/β-PbO2 anode achieving boosted electrocatalytic oxidation of As (III), Journal of Hazardous Materials, 2022, 430, 128449.

  49. Peng Liu, Zhikai Li, Kuan Deng, Xingbin Lv, Wen Tian, Hongjiao Li, Shuai Tan, Shaojun Yuan, Junyi Ji, Hierarchical BiVO4/Cu(OH)2 nanocone/nanowire membrane with environmental durability and electro-/photo-cleaning capability for oil/water separation, Surface & Coatings Technology, 2022, 434, 128175.

  50. Ji Li, Ruixi Gao, Yuan Wang, Tian C Zhang, Shaojun Yuan*, Superhydrophobic palmitic acid modified Cu(OH)2/CuS nanocomposite-coated copper foam for efficient separation of oily wastewater, Colloids and Surfaces A: Physicochemical and Engineering Aspects, 2022, 637, 128249.

  51. Yanbo Deng, Pengfei Tian, Shijie Liu, Huaqiang He, Yuan Wang, Like Ouyang, Shaojun Yuan*, Enhanced catalytic performance of atomically dispersed Pd on Pr-doped CeO2 nanorod in CO oxidation, Journal of Hazardous Materials, 2022, 426, 127793.

  52. Shijie Liu, Yanbo Deng, Lian Fu, Lijia Huang, Like Ouyang, Shaojun Yuan, Understanding the role of boron on the interface modulation of the Pd/TiO2 catalyst for direct synthesis of H2O2, ACS Sustainable Chemistry & Engineering, 2022, 10 (10), 3264-3275

  53. Hui Liu, Wangchen Huo, Tian C Zhang, Like Ouyang, Shaojun Yuan*, Photocatalytic removal of tetracycline by a Z-scheme heterojunction of bismuth oxyiodide/exfoliated g-C3N4: performance, mechanism, and degradation pathway, Materials Today Chemistry, 2022, 23, 100729.

  54. Huaqiang He, Tian C Zhang, Like Ouyang, Shaojun Yuan, Superwetting and photocatalytic Ag2O/TiO2@ CuC2O4 nanocomposite-coated mesh membranes for oil/water separation and soluble dye removal, Materials Today Chemistry, 2022, 23, 100717.

  55. Yuan Wang, Jianfei Xiao, Hanzhi Wang, Tian C Zhang, Shaojun Yuan*, Binary doping of nitrogen and phosphorus into porous carbon: A novel di-functional material for enhancing CO2 capture and super-capacitance, Journal of Materials Science & Technology, 2022, 99, 73-81.

  56. Yufang Zhang, Jianfei Xiao, Tian C Zhang, Like Ouyang, Shaojun Yuan*, Synthesis of CuSiO3-loaded P-doped porous biochar derived from phytic acid-activated lemon peel for enhanced adsorption of NH3, Separation and Purification Technology, 2022, 283, 120179.

  57. Quyun Chen, Tian C Zhang, Like Ouyang, Shaojun Yuan*, Single-step hydrothermal synthesis of biochar from H3PO4-activated lettuce waste for efficient adsorption of Cd (II) in aqueous solution, 2022, Molecules, 27 (1), 269.

  58. Jianfei Xiao, Yuan Wang, Tian C Zhang, Like Ouyang, Shaojun Yuan*, Phytic acid-induced self-assembled chitosan gel-derived N,P-co-doped porous carbon for high-performance CO2 capture and supercapacitor, Journal of Power Sources, 2022, 517, 230727.


 

 

 


 



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